n_TOF Collaboration(Lederer, C. et al), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2013). Neutron Capture Cross Section of Unstable Ni-63: Implications for Stellar Nucleosynthesis. Phys. Rev. Lett., 110(2), 022501–5pp.
Abstract: The Ni-63(n, gamma) cross section has been measured for the first time at the neutron time-of-flight facility n_TOF at CERN from thermal neutron energies up to 200 keV. In total, capture kernels of 12 (new) resonances were determined. Maxwellian averaged cross sections were calculated for thermal energies from kT = 5-100 keV with uncertainties around 20%. Stellar model calculations for a 25M(circle dot) star show that the new data have a significant effect on the s-process production of Cu-63, Ni-64, and Zn-64 in massive stars, allowing stronger constraints on the Cu yields from explosive nucleosynthesis in the subsequent supernova.
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Guerrero, C., Cano-Ott, D., Mendoza, E., Tain, J. L., Algora, A., Berthoumieux, E., et al. (2012). Monte Carlo simulation of the n_TOF Total Absorption Calorimeter. Nucl. Instrum. Methods Phys. Res. A, 671, 108–117.
Abstract: The n_TOF Total Absorption Calorimeter (TAC) is a 4 pi BaF2 segmented detector used at CERN for measuring neutron capture cross-sections of importance for the design of advanced nuclear reactors. This work presents the simulation code that has been developed in GEANT4 for the accurate determination of the detection efficiency of the TAC for neutron capture events. The code allows to calculate the efficiency of the TAC for every neutron capture state, as a function of energy, crystal multiplicity, and counting rate. The code includes all instrumental effects such as the single crystal detection threshold and energy resolution, finite size of the coincidence time window, and signal pile-up. The results from the simulation have been validated with experimental data for a large set of electromagnetic de-excitation patterns: beta-decay of well known calibration sources, neutron capture reactions in light nuclei with well known level schemes like Ti-nat, reference samples used in (n,gamma) measurements like Au-197 and experimental data from an actinide sample like Pu-240. The systematic uncertainty in the determination of the detection efficiency has been estimated for all the cases. As a representative example, the accuracy reached for the case of Au-197(n,gamma) ranges between 0.5% and 2%, depending on the experimental and analysis conditions. Such a value matches the high accuracy required for the nuclear cross-section data needed in advanced reactor design.
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n_TOF Collaboration(Mosconi, M. et al), Domingo-Pardo, C., & Tain, J. L. (2010). Neutron physics of the Re/Os clock. I. Measurement of the (n, gamma) cross sections of Os-186,Os-187,Os-188 at the CERN n_TOF facility. Phys. Rev. C, 82(1), 015802–10pp.
Abstract: The precise determination of the neutron capture cross sections of Os-186 and Os-187 is important to define the s-process abundance of Os-187 at the formation of the solar system. This quantity can be used to evaluate the radiogenic component of the abundance of Os-187 due to the decay of the unstable Re-187 (t(1/2) = 41.2 Gyr) and from this to infer the time duration of the nucleosynthesis in our galaxy (Re/Os cosmochronometer). The neutron capture cross sections of Os-186, Os-187, and Os-188 have been measured at the CERN n_TOF facility from 1 eV to 1 MeV, covering the entire energy range of astrophysical interest. The measurement has been performed by time-of-flight technique using isotopically enriched samples and two C6D6 scintillation detectors for recording the prompt. rays emitted in the capture events. Maxwellian averaged capture cross sections have been determined for thermal energies between kT = 5 and 100 keV corresponding to all possible s-process scenarios. The estimated uncertainties for the values at 30 keV are 4.1, 3.3, and 4.7% for Os-186, Os-187, and Os-188, respectively.
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n_TOF Collaboration(Wright, T. et al), Domingo-Pardo, C., Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2017). Measurement of the U-238(n,gamma) cross section up to 80 keV with the Total Absorption Calorimeter at the CERN n_TOF facility. Phys. Rev. C, 96(6), 064601–11pp.
Abstract: The radiative capture cross section of a highly pure (99.999%), 6.125(2) grams and 9.56(5) x 10(-4) atoms/barn areal density U-238 sample has been measured with the Total Absorption Calorimeter (TAC) in the 185 m flight path at the CERN neutron time-of-flight facility n_TOF. This measurement is in response to the NEA High Priority Request list, which demands an accuracy in this cross section of less than 3% below 25 keV. These data have undergone careful background subtraction, with special care being given to the background originating from neutrons scattered by the 238U sample. Pileup and dead-time effects have been corrected for. The measured cross section covers an energy range between 0.2 eV and 80 keV, with an accuracy that varies with neutron energy, being better than 4% below 25 keV and reaching at most 6% at higher energies.
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n_TOF Collaboration(Belloni, F. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Measurement of the neutron-induced fission cross-section of Am-243 relative to U-235 from 0.5 to 20 MeV. Eur. Phys. J. A, 47(12), 160–8pp.
Abstract: The ratio of the neutron-induced fission cross-sections of Am-243 and U-235 was measured in the energy range from 0.5 to 20 MeV with uncertainties of approximate to 4%. The experiment was performed at the CERN n_TOF facility using a fast ionization chamber. With the good counting statistics that could be achieved thanks to the high instantaneous flux and the low backgrounds, the present results are useful for resolving discrepancies in previous data sets and are important for future reactors with improved fuel burn-up.
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