Abstract: A low-lying state in In-131(82), the one-proton hole nucleus with respect to double magic Sn-132, was observed by its gamma decay to the I-pi 1/2(-) beta-emitting isomer. We identify the new state at an excitation energy of E-x = 1353 keV, which was populated both in the beta decay of Cd-131(83) and after beta-delayed neutron emission from Cd-132(84), as the previously unknown pi p(3/2) single-hole state with respect to the Sn-132 core. Exploiting this crucial new experimental information, shell-model calculations were performed to study the structure of experimentally inaccessible N = 82 isotones below Sn-132. The results evidence a surprising absence of proton subshell closures along the chain of N = 82 isotones. The consequences of this finding for the evolution of the N = 82 shell gap along the r-process path are discussed.

Abstract: A new isomer with a half-life of 23.0(8) ms has been identified at 2406 keV in Pd-126 and is proposed to have a spin and parity of 10(+) with a maximally aligned configuration comprising two neutron holes in the 1h(11/2) orbit. In addition to an internal-decay branch through a hindered electric octupole transition, beta decay from the long-lived isomer was observed to populate excited states at high spins in Ag-126. The smaller energy difference between the 10(+) and 7(-) isomers in Pd-126 than in the heavier N = 80 isotones can be interpreted as being ascribed to the monopole shift of the 1h(11/2) neutron orbit. The effects of the monopole interaction on the evolution of single-neutron energies below Sn-132 are discussed in terms of the central and tensor forces.

Abstract: Background: beta-delayed multiple neutron emission has been observed for some nuclei with A <= 100 being the Rb-100 the heaviest beta 2n emitter measured to date. So far only 25 P-2n values have been determined for the approximate to 300 nuclei that may decay in this way. Accordingly it is of interest to measure P-2n values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such a measurement for nuclei with A > 100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the r-process and safety inputs for nuclear reactors. Purpose: To determine for the first time the two-neutron branching ratio the P-2n value for Sb-136 through a direct neutron measurement and to provide precise P-1n values for Sb-136 and Te-136. Method: A pure beam of each isotope of interest was provided by the JYFLTRAP Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility of the University of Jyvaskyla Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point after the tape to register the beta decays and the BELEN detector based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the beta- and neutron-growth-and-decay curves and the beta-one-neutron and beta-two-neutron time correlations which allowed us the determination of the neutron branching ratios. Results: The P-2n value of Sb-136 was found to be 0.14(3)% and the measured P-1n values for Sb-136 and Te-136 were found to be 32.2(15)% and 1.47(6)% respectively. Conclusions: The measured P-2n value is a factor 44 smaller than predicted by the finite-range droplet model plus the quasiparticle random-phase approximation (FRDM+QRPA) model used for r-process calculations.