Abstract: Background: The Z = 50 shell closure, near N = 82, is unique in the sense that it is the only shell closure with the spin-orbit partner orbitals, pi g(9/2) and pi g(7/2), enclosing the magic gap. The interaction of the proton hole/particle in the above-mentioned orbitals with neutrons in the nu h(11)(/2) orbital is an important prerequisite to the understanding of the nuclear structure near N = 82 and the nu pi interaction. Purpose: To explore the structural similarity between the high-spin isomeric states in In (Z = 49), Sn (Z = 50), and Sb (Z = 51) isotopes from a microscopic point of view. In addition, to understand the role of a proton hole or particle in the spin-orbit partner orbitals, pi g(9/2) and pi g(7/2), respectively, with neutron holes in the nu h(11)(/2) orbital on these aforementioned isomers. Methods: The fusion and transfer induced fission reaction Be-9(U-238, f) with 6.2 MeV/u beam energy, using a unique setup consisting of AGATA, VAMOS ++, and EXOGAM detectors, was used to populate through the fission process and study the neutron-rich In-119,In-121 isotopes. This setup enabled the prompt-delayed gamma-ray spectroscopy of isotopes in the time range of 100 ns-200 μs. Results: In the odd-A In-119,In-121 isotopes, indications of a short half-life 19/2(-) isomeric state, in addition to the previously known 25/2(+) isomeric state, were observed from the present data. Further, new prompt transitions above the 25/2(+) isomer in In-121 were identified along with reevaluation of its half-life. Conclusions: The experimental data were compared with the theoretical results obtained in the framework of large-scale shell-model calculations in a restricted model space. The <pi g(9/2)nu h(11/2); I vertical bar H vertical bar pi g(9/2) nu h(11/2);I > two-body matrix elements of residual interaction were modified to explain the excitation energies and the B(E2) transition probabilities in the neutron-rich In isotopes. The (i) decreasing trend of E(29/2(+))-E(25/2(+)) in odd-In (with dominant configuration pi g(9/)(2)(-1) nu h(11/2)(-2) and maximum aligned spin of 29/2+) and (ii) increasing trend of E(27/2(+)) – E(23/2(+)) in odd-Sb (with dominant configuration pi g(7/)(2)(+1) nu h(11/2)(-2) and maximum aligned spin of 27/2(+)) with increasing neutron number could be understood as a consequence of hole-hole and particle-hole interactions, respectively.

Abstract: Level lifetimes of the yrast (5/2(-)) to 13/2(-) states in the neutron-rich nucleus Ti-53, produced in a multinucleon-transfer reaction, have been measured for the first time. The recoil distance Doppler-shift method was employed and lifetimes of the excited states were extracted by a lineshape analysis aided by GEANT4-based Monte-Carlo simulations. The experiment was performed at the Grand Accelerateur National d'Ions Lourds facility in Caen, France, by using the Advanced Gamma Tracking Array for the gamma-ray detection coupled to the large-acceptance variable mode spectrometer for an event-by-event particle identification and the Cologne plunger for deep-inelastic reactions. Reduced transition probabilities, deduced from the lifetimes, give new information on the nuclear structure of Ti-53, and are used to benchmark different shell-model calculations using established interactions in the f p shell.

Abstract: Background: The heaviest T-z = 0 doubly-magic nucleus, Sn-100, and the neighboring nuclei offer unique opportunities to investigate the properties of nuclear interaction. For instance, the structure of light-Sn nuclei has been shown to be affected by the delicate balance between nuclear-interaction components, such as pairing and quadrupole correlations. From Cd to Te, many common features and phenomena have been observed experimentally along the isotopic chains, leading to theoretical studies devoted to a more general and comprehensive study of the region. In this context, having only two proton holes in the Z = 50 shell, the Cd isotopes are expected to present properties similar to those found in the Sn isotopic chain. Purpose: The aim of this work was to measure lifetimes of excited states in neutron-deficient nuclei in the vicinity of Sn-100. Methods: The neutron-deficient nuclei in the N approximate to Z approximate to 50 region were populated using a multinucleon transfer reaction with a Cd-106 beam and a Mo-92 target. The beamlike products were identified by the VAMOS++ spectrometer, while the gamma rays were detected using the AGATA array. Lifetimes of excited states were determined using the recoil distance Doppler-shift method, employing the Cologne differential plunger. Results: Lifetimes of low-lying states were measured in the even-mass Cd-102-(108) isotopes. In particular, multiple states with excitation energy up to MeV, belonging to various bands, were populated in approximate to 3 Cd-106 via inelastic scattering. The transition strengths corresponding to the measured lifetimes were compared with those resulting from state-of-the-art beyond-mean-field calculations using the symmetry-conserving configuration-mixing approach. Conclusions: Despite the similarities in the electromagnetic properties of the low-lying states, there is a fundamental structural difference between the ground-state bands in the Z = 48 and Z = 50 isotopes. The comparison between experimental and theoretical results revealed a rotational character of the Cd nuclei, which have prolate-deformed ground states with beta(2) approximate to 0.2. At this deformation Z = 48 becomes a closed-shell configuration, which is favored with respect to the spherical one.

Abstract: The structure of As-83,As- 85, and As-87 have been studied in fusion-fission reaction( 238)U+9Be. Fission fragments were identified in mass and atomic number using the VAMOS++ spectrometer and the coincident gamma rays were detected in the gamma-ray tracking array AGATA. New transitions in 83As and 85As are reported and placed in the level schemes. A level scheme of the excited states in 87As is proposed for the first time. The data are interpreted in frame of large-scale shell-model calculations, SU3 symmetries, and beyond mean-field frameworks. A spherical regime at magic number N = 50 is predicted and the location of the proton g9/2 orbital is proposed for the first time. Development of collectivity in a prolate deformed, gamma-soft regime in the open shell cases 85As and 87As, most neutron-rich isotopes beyond N = 50, is concluded. Data and theoretical calculations give confidence to a relatively high extrapolated excitation energy about 4 MeV of the 9/2+ state in 79Cu, one proton above 78Ni.

Abstract: Prompt.-ray spectroscopy of the neutron-rich Kr-96, produced in transfer-and fusion-induced fission reactions, has been performed using the combination of the Advanced Gamma Tracking Array and the VAMOS + +spectrometer. A second excited state, assigned to J pi = 4(+), is observed for the first time, and a previously reported level energy of the first 2+ excited state is confirmed. The measured energy ratio R-4/2 = E(4(+))/E(2(+)) = 2.12(1) indicates that this nucleus does not show a well-developed collectivity contrary to that seen in heavier N = 60 isotones. This new measurement highlights an abrupt transition of the degree of collectivity as a function of the proton number at Z = 36, of similar amplitude to that observed at N = 60 at higher Z values. A possible reason for this abrupt transition could be related to the insufficient proton excitations in the g(9/2), d(5/2), and s(1/2) orbitals to generate strong quadrupole correlations or to the coexistence of competing different shapes. An unexpected continuous decrease of R-4/2 as a function of the neutron number up to N = 60 is also evidenced. This measurement establishes the Kr isotopic chain as the low-Z boundary of the island of deformation for N = 60 isotones. A comparison with available theoretical predictions using different beyond mean-field approaches shows that these models fail to reproduce the abrupt transitions at N = 60 and Z = 36.