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Guadilla, V. et al; Tain, J.L.; Algora, A.; Agramunt, J.; Jordan, D.; Monserrate, M.; Montaner-Piza, A.; Orrigo, S.E.A.; Rubio, B.; Valencia, E. |
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Title |
Determination of beta-decay ground state feeding of nuclei of importance for reactor applications |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal  |
Phys. Rev. C |
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Volume |
102 |
Issue |
6 |
Pages |
064304 - 12pp |
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Keywords |
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Abstract |
In beta-decay studies the determination of the decay probability to the ground state (g.s.) of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed gamma-ray emission. In this work we revisit the 4 pi gamma – beta method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the beta-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large g.s. branches. The method is relevant for nuclear structure studies as well. Pertinent formulas are revised and extended to the special case of beta-delayed neutron emitters, and the robustness of the method is demonstrated with synthetic data. We apply it to a number of measured decays that serve as test cases and discuss the features of the method. Finally, we obtain g.s. feeding intensities with reduced uncertainty for four relevant decays that will allow future improvements in antineutrino spectrum and decay heat calculations using the summation method. |
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Address |
[Guadilla, V; Tain, J. L.; Algora, A.; Agramunt, J.; Jordan, D.; Monserrate, M.; Montaner-Piza, A.; Orrigo, S. E. A.; Rubio, B.; Valencia, E.] Univ Valencia, Inst Fis Corpuscular, CSIC, E-46071 Valencia, Spain |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
ISBN |
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Expedition |
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Conference |
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Notes |
WOS:000595153500001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4626 |
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Author |
Guadilla, V. et al; Algora, A.; Tain, J.L.; Agramunt, J.; Jordan, D.; Monserrate, M.; Montaner-Piza, A.; Nacher, E.; Orrigo, S.E.A.; Rubio, B.; Valencia, E. |
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Title |
Total absorption gamma-ray spectroscopy of the ss decays of Y-96gs,Y-m |
Type |
Journal Article |
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Year |
2022 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
106 |
Issue |
1 |
Pages |
014306 - 14pp |
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Keywords |
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Abstract |
The ss decays of the ground state (gs) and isomeric state (m) of Y-96 have been studied with the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8(+) isomeric state from the 0(-) ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The ss-intensity distributions of both decays have been independently determined. In the analyses the deexcitation of the 1581.6 keV level in Zr-96, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the ss-detector efficiency, influencing the ss-intensity distribution obtained. Our results for Y-96gs (0(-)) confirm the large ground state to ground state ss-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to 96.6(-2.1)(+0.3) % of the total ss intensity. Given that the decay of Y-96gs is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of Y-96m (8(+)), previously undetected ss intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption gamma-ray spectroscopy measurements of ss decays with highly fragmented deexcitation patterns. Y-96m (8(+)) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average ss and gamma energies differ significantly from the previous values in evaluated databases. The discrepancy is far above the previously quoted uncertainties. Finally, we also report on the successful implementation of an innovative total absorption gamma-ray spectroscopy analysis of the module-multiplicity gated spectra, as a first proof of principle to distinguish between decaying states with very different spin-parity values. |
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Address |
[Guadilla, V; Le Meur, L.; Fallot, M.; Briz, J. A.; Estienne, M.; Giot, L.; Porta, A.; Cucoanes, A.; Shiba, T.; Zakari-Issoufou, A-A] Univ Nantes, Subatech, IMT Atlantique, CNRS IN2P3, F-44307 Nantes, France, Email: vguadilla@fuw.edu.pl |
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Amer Physical Soc |
Place of Publication |
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English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000832364800001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5313 |
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Author |
Grieger, M.; Hensel, T.; Agramunt, J.; Bemmerer, D.; Degering, D.; Dillmann, I.; Fraile, L.M.; Jordan, D.; Koster, U.; Marta, M.; Muller, S.E.; Szucs, T.; Tain, J.L.; Zuber, K. |
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Title |
Neutron flux and spectrum in the Dresden Felsenkeller underground facility studied by moderated He-3 counters |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review D |
Abbreviated Journal |
Phys. Rev. D |
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Volume |
101 |
Issue |
12 |
Pages |
123027 - 15pp |
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Keywords |
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Abstract |
Ambient neutrons may cause significant background for underground experiments. Therefore, it is necessary to investigate their flux and energy spectrum in order to devise a proper shielding. Here, two sets of altogether ten moderated He-3 neutron counters are used for a detailed study of the ambient neutron background in tunnel IV of the Felsenkeller facility, underground below 45 m of rock in Dresden/Germany. One of the moderators is lined with lead and thus sensitive to neutrons of energies higher than 10 MeV. For each He-3 counter moderator assembly, the energy-dependent neutron sensitivity was calculated with the FLUKA code. The count rates of the ten detectors were then fitted with the MAXED and GRAVEL packages. As a result, both the neutron energy spectrum from 10(-9) to 300 MeV and the flux integrated over the same energy range were determined experimentally. The data show that at a given depth, both the flux and the spectrum vary significantly depending on local conditions. Energy-integrated fluxes of (0.61 +/- 0.05), (1.96 +/- 0.15), and (4.6 +/- 0.4) x 10(-4) cm(-2) s(-1), respectively, are measured for three sites within Felsenkeller tunnel IV which have similar muon flux but different shielding wall configurations. The integrated neutron flux data and the obtained spectra for the three sites are matched reasonably well by FLUKA Monte Carlo calculations that are based on the known muon flux and composition of the measurement room walls. |
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Address |
[Grieger, M.; Hensel, T.; Bemmerer, D.; Mueller, S. E.; Szuecs, T.] Helmholtz Zentrum Dresden Rossendorf HZDR, D-01328 Dresden, Germany, Email: d.bemmerer@hzdr.de |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1550-7998 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000542517900002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4442 |
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| Permanent link to this record |
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Author |
Algora, A. et al; Jordan, D.; Tain, J.L.; Rubio, B.; Agramunt, J.; Perez-Cerdan, A.B.; Molina, F.; Caballero, L.; Nacher, E. |
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Title |
Reactor Decay Heat in Pu-239: Solving the gamma Discrepancy in the 4-3000-s Cooling Period |
Type |
Journal Article |
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Year |
2010 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
105 |
Issue |
20 |
Pages |
202501 - 4pp |
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Keywords |
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Abstract |
The beta feeding probability of Tc-102,Tc- 104,Tc- 105,Tc- 106,Tc- 107, Mo-105, and Nb-101 nuclei, which are important contributors to the decay heat in nuclear reactors, has been measured using the total absorption technique. We have coupled for the first time a total absorption spectrometer to a Penning trap in order to obtain sources of very high isobaric purity. Our results solve a significant part of a long-standing discrepancy in the gamma component of the decay heat for Pu-239 in the 4-3000 s range. |
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Address |
[Algora, A.; Jordan, D.; Tain, J. L.; Rubio, B.; Agramunt, J.; Perez-Cerdan, A. B.; Molina, F.; Caballero, L.; Nacher, E.] Univ Valencia, IFIC, CSIC, Valencia, Spain, Email: algora@ific.uv.es |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0031-9007 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
ISI:000283927700004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
328 |
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Author |
Fallot, M.; Cormon, S.; Estienne, M.; Algora, A.; Bui, V.M.; Cucoanes, A.; Elnimr, M.; Giot, L.; Jordan, D.; Martino, J.; Onillon, A.; Porta, A.; Pronost, G.; Remoto, A.; Tain, J.L.; Yermia, F.; Zakari-Issoufou, A.A. |
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Title |
New Antineutrino Energy Spectra Predictions from the Summation of Beta Decay Branches of the Fission Products |
Type |
Journal Article |
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Year |
2012 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
109 |
Issue |
20 |
Pages |
202504 - 5pp |
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Keywords |
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Abstract |
In this Letter, we study the impact of the inclusion of the recently measured beta decay properties of the Tc-102;104;105;106;107, Mo-105, and Nb-101 nuclei in an updated calculation of the antineutrino energy spectra of the four fissible isotopes U-235,U-238 and Pu-239,Pu-241. These actinides are the main contributors to the fission processes in pressurized water reactors. The beta feeding probabilities of the above-mentioned Tc, Mo, and Nb isotopes have been found to play a major role in the gamma component of the decay heat of Pu-239, solving a large part of the gamma discrepancy in the 4-3000 s range. They have been measured by using the total absorption technique, insensitive to the pandemonium effect. The calculations are performed by using the information available nowadays in the nuclear databases, summing all the contributions of the beta decay branches of the fission products. Our results provide a new prediction of the antineutrino energy spectra of U-235, Pu-239,Pu-241, and, in particular, U-238 for which no measurement has been published yet. We conclude that new total absorption technique measurements are mandatory to improve the reliability of the predicted spectra. |
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Address |
[Fallot, M.; Cormon, S.; Estienne, M.; Bui, V. M.; Cucoanes, A.; Elnimr, M.; Giot, L.; Martino, J.; Onillon, A.; Porta, A.; Pronost, G.; Remoto, A.; Yermia, F.; Zakari-Issoufou, A. -A.] Univ Nantes, Ecole Mines Nantes, CNRS, IN2P3,SUBATECH, F-44307 Nantes, France |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0031-9007 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000310991700009 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1250 |
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| Permanent link to this record |
