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n_TOF Collaboration (Mendoza, E. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Measurement and analysis of the Am-243 neutron capture cross section at the n_TOF facility at CERN |
Type |
Journal Article |
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Year |
2014 |
Publication |
Physical Review C |
Abbreviated Journal  |
Phys. Rev. C |
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Volume |
90 |
Issue |
3 |
Pages |
034608 - 16pp |
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Abstract |
Background: The design of new nuclear reactors and transmutation devices requires to reduce the present neutron cross section uncertainties of minor actinides. Purpose: Improvement of the Am-243(n, gamma) cross section uncertainty. Method: The Am-243(n, gamma) cross section has been measured at the n_TOF facility at CERN with a BaF2 total absorption calorimeter, in the energy range between 0.7 eV and 2.5 keV. Results: The Am-243(n, gamma) cross section has been successfully measured in the mentioned energy range. The resolved resonance region has been extended from 250 eV up to 400 eV. In the unresolved resonance region our results are compatible with one of the two incompatible capture data sets available below 2.5 keV. The data available in EXFOR and in the literature have been used to perform a simple analysis above 2.5 keV. Conclusions: The results of this measurement contribute to reduce the Am-243(n, gamma) cross section uncertainty and suggest that this cross section is underestimated up to 25% in the neutron energy range between 50 eV and a few keV in the present evaluated data libraries. |
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[Mendoza, E.; Cano-Ott, D.; Guerrero, C.; Alvarez-Velarde, F.; Balibrea, J.; Gonzalez-Romero, E.; Martinez, T.; Villamarin, D.; Vicente, M. C.] CIEMAT, E-28040 Madrid, Spain |
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Amer Physical Soc |
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0556-2813 |
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Notes |
WOS:000341912100005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1935 |
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Molina, F. et al; Rubio, B.; Agramunt, J.; Algora, A.; Domingo-Pardo, C.; Gadea, A.; Tain, J.L. |
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Title |
T-z =-1 -> 0 beta decays of Ni-54, Fe-50, Cr-46, and Ti-42 and comparison with mirror (He-3,t) measurements |
Type |
Journal Article |
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Year |
2015 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
91 |
Issue |
1 |
Pages |
014301 - 19pp |
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Abstract |
We have studied the beta decay of the T-z = -1, f(7/2) shell nuclei Ni-54, Fe-50, Cr-46, and Ti-42 produced in fragmentation reactions. The proton separation energies in the daughter T-z = 0 nuclei are relatively large (approximate to 4-5 MeV) so studies of the. rays are essential. The experiments were performed at GSI as part of the Stopped-beam campaign with the RISING setup consisting of 15 Euroball Cluster Ge detectors. From the newly obtained high precision beta-decay half-lives, excitation energies, and beta branching ratios, we were able to extract Fermi and Gamow-Teller transition strengths in these beta decays. With these improved results it was possible to compare in detail the Gamow-Teller (GT) transition strengths observed in beta decay including a sensitivity limit with the strengths of the T-z = +1 to T-z = 0 transitions derived from high resolution (He-3,t) reactions on the mirror target nuclei at RCNP, Osaka. The accumulated B(GT) strength obtained from both experiments looks very similar although the charge exchange reaction provides information on a broader energy range. Using the “merged analysis” one can obtain a full picture of the B(GT) over the full Q(beta) range. Looking at the individual transitions some differences are observed, especially for the weak transitions. Their possible origins are discussed. |
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Address |
[Molina, F.; Rubio, B.; Agramunt, J.; Algora, A.; Domingo-Pardo, C.; Gadea, A.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46071 Valencia, Spain, Email: berta.rubio@ific.uv.es |
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Amer Physical Soc |
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0556-2813 |
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WOS:000347924300002 |
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no |
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yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2087 |
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n_TOF Collaboration (Paradela, C. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
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Title |
High-accuracy determination of the U-238/U-235 fission cross section ratio up to approximate to 1 GeV at n_TOF at CERN |
Type |
Journal Article |
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Year |
2015 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
91 |
Issue |
2 |
Pages |
024602 - 11pp |
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Abstract |
The U-238 to U-235 fission cross section ratio has been determined at nTOF up to approximate to 1 GeV, with two different detection systems, in different geometrical configurations. A total of four datasets has been collected and compared. They are all consistent to each other within the relative systematic uncertainty of 3-4%. The data collected at nTOF have been suitably combined to yield a unique fission cross section ratio as a function of neutron energy. The result confirms current evaluations up to 200 MeV. Good agreement is also observed with theoretical calculations based on the INCL++ /Gemini++ combination up to the highest measured energy. The n_TOF results may help solve a long-standing discrepancy between the two most important experimental datasets available so far above 20 MeV, while extending the neutron energy range for the first time up to approximate to 1 GeV. |
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Address |
[Paradela, C.; Tarrio, D.; Leal-Cidoncha, E.; Duran, I.; Alvarez, H.] Univ Santiago de Compostela, Santiago De Compostela, Spain, Email: nicola.colonna@ba.infn.it |
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Amer Physical Soc |
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0556-2813 |
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Notes |
WOS:000350174000004 |
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no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2139 |
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n_TOF Collaboration (Diakaki, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron-induced fission cross section of Np-237 in the keV to MeV range at the CERN n_TOF facility |
Type |
Journal Article |
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Year |
2016 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
93 |
Issue |
3 |
Pages |
034614 - 12pp |
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Abstract |
The neutron-induced fission cross section of Np-237 was experimentally determined at the high-resolution and high-intensity facility n_TOF, at CERN, in the energy range 100 keV to 9 MeV, using the U-235(n, f) and U-238(n, f) cross section standards below and above 2 MeV, respectively. A fast ionization chamber was used in order to detect the fission fragments from the reactions and the targets were characterized as far as their mass and homogeneity are concerned by means of a spectroscopy and Rutherford backscattering spectroscopy respectively. Theoretical calculations within the Hauser-Feshbach formalism have been performed, employing the EMPIRE code, and the model parameters were tuned in order to successfully reproduce the experimental fission cross-sectional data and simultaneously all the competing reaction channels. |
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Address |
[Diakaki, M.; Aerts, G.; Andriamonje, S.; Berthoumieux, E.] CEA Saclay, DSM, F-91191 Gif Sur Yvette, France, Email: maria.diakaki@cea.fr |
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Amer Physical Soc |
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2469-9985 |
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Notes |
WOS:000372415600004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2591 |
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Author |
n_TOF Collaboration (Mingrone, F. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
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Title |
Neutron capture cross section measurement of U-238 at the CERN n_TOF facility in the energy region from 1 eV to 700 keV |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
95 |
Issue |
3 |
Pages |
034604 - 14pp |
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Abstract |
The aim of this work is to provide a precise and accurate measurement of the U-238(n,gamma) reaction cross section in the energy region from 1 eV to 700 keV. This reaction is of fundamental importance for the design calculations of nuclear reactors, governing the behavior of the reactor core. In particular, fast reactors, which are experiencing a growing interest for their ability to burn radioactive waste, operate in the high energy region of the neutron spectrum. In this energy region most recent evaluations disagree due to inconsistencies in the existing measurements of up to 15%. In addition, the assessment of nuclear data uncertainty performed for innovative reactor systems shows that the uncertainty in the radiative capture cross section of U-238 should be further reduced to 1-3% in the energy region from 20 eV to 25 keV. To this purpose, addressed by the Nuclear Energy Agency as a priority nuclear data need, complementary experiments, one at the GELINA and two at the nTOF facility, were proposed and carried out within the 7th Framework Project ANDES of the European Commission. The results of one of these U-238(n, gamma) measurements performed at the nTOF CERN facility are presented in this work. The gamma-ray cascade following the radiative neutron capture has been detected exploiting a setup of two C6D6 liquid scintillators. Resonance parameters obtained from this work are on average in excellent agreement with the ones reported in evaluated libraries. In the unresolved resonance region, this work yields a cross section in agreement with evaluated libraries up to 80 keV, while for higher energies our results are significantly higher. |
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Address |
[Mingrone, F.; Berthoumieux, E.; Brugger, M.; Calviani, M.; Cerutti, F.; Chiaveri, E.; Chin, M.; Guerrero, C.; Hernandez-Prieto, A.; Kadi, Y.; Losito, R.; Rubbia, C.; Tsinganis, A.; Vlachoudis, V.] CERN, European Org Nucl Res, Geneva, Switzerland, Email: federica.mingrone@cern.ch |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Notes |
WOS:000396022500002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3030 |
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Author |
PreSPEC and AGATA Collaborations (Ralet, D. et al); Domingo-Pardo, C.; Gadea, A.; Huyuk, T. |
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Title |
Lifetime measurement of neutron-rich even-even molybdenum isotopes |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
95 |
Issue |
3 |
Pages |
034320 - 11pp |
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Keywords |
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Abstract |
Background: In the neutron-rich A approximate to 100 mass region, rapid shape changes as a function of nucleon number as well as coexistence of prolate, oblate, and triaxial shapes are predicted by various theoretical models. Lifetime measurements of excited levels in the molybdenum isotopes allow the determination of transitional quadrupole moments, which in turn provides structural information regarding the predicted shape change. Purpose: The present paper reports on the experimental setup, the method that allowed one to measure the lifetimes of excited states in even-even molybdenum isotopes from mass A = 100 up to mass A = 108, and the results that were obtained. Method: The isotopes of interest were populated by secondary knock-out reaction of neutron-rich nuclei separated and identified by the GSI fragment separator at relativistic beam energies and detected by the sensitive PreSPEC-AGATA experimental setup. The latter included the Lund-York-Cologne calorimeter for identification, tracking, and velocity measurement of ejectiles, and AGATA, an array of position sensitive segmented HPGe detectors, used to determine the interaction positions of the gamma ray enabling a precise Doppler correction. The lifetimes were determined with a relativistic version of the Doppler-shift-attenuation method using the systematic shift of the energy after Doppler correction of a gamma-ray transition with a known energy. This relativistic Doppler-shift-attenuation method allowed the determination of mean lifetimes from 2 to 250 ps. Results: Even-even molybdenum isotopes from mass A = 100 to A = 108 were studied. The decays of the low-lying states in the ground-state band were observed. In particular, two mean lifetimes were measured for the first time: tau = 29.7(-9.1)(+11.3) ps for the 4(+) state of Mo-108 and tau = 3.2(-0.7)(+ 0.7) ps for the 6(+) state of Mo-102. Conclusions: The reduced transition strengths B(E2), calculated from lifetimes measured in this experiment, compared to beyond-mean-field calculations, indicate a gradual shape transition in the chain of molybdenum isotopes when going from A = 100 to A = 108 with a maximum reached at N = 64. The transition probabilities decrease for Mo-108 which may be related to its well-pronounced triaxial shape indicated by the calculations. |
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Address |
[Ralet, D.; Cortes, M. L.; Gregor, E.; Guastalla, G.; Givechev, A.; Habermann, T.; Louchart-Henning, C.; Merchan, E.; Pietralla, N.; Reese, M.; Singh, P. P.; Stahl, C.] Tech Univ Darmstadt, Inst Kernphys, D-64289 Darmstadt, Germany, Email: ralet@csnsm.in2p3.fr |
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Amer Physical Soc |
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2469-9985 |
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Notes |
WOS:000399143200002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3045 |
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Ong, W.J. et al; Domingo-Pardo, C. |
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Title |
Low-lying level structure of Cu-56 and its implications for the rp process |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
95 |
Issue |
5 |
Pages |
055806 - 8pp |
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Keywords |
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Abstract |
The low-lying energy levels of proton-rich Cu-56 have been extracted using in-beam gamma-ray spectroscopy with the state-of-the-art gamma-ray tracking array GRETINA in conjunction with the S800 spectrograph at the National Superconducting Cyclotron Laboratory at Michigan State University. Excited states in Cu-56 serve as resonances in the Ni-55(p,gamma)Cu-56 reaction, which is a part of the rp process in type-I x-ray bursts. To resolve existing ambiguities in the reaction Q value, a more localized isobaric multiplet mass equation (IMME) fit is used, resulting in Q = 639 +/- 82 keV. We derive the first experimentally constrained thermonuclear reaction rate for Ni-55(p,.) Cu-56. We find that, with this newrate, the rp processmay bypass the (56)Niwaiting point via the Ni-55(p,gamma) reaction for typical x-ray burst conditions with a branching of up to similar to 40%. We also identify additional nuclear physics uncertainties that need to be addressed before drawing final conclusions about the rp-process reaction flow in the Ni-56 region. |
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[Ong, W. -J.; Langer, C.; Montes, F.; Bazin, D.; Brown, B. A.; Browne, J.; Cyburt, R.; Deleeuw, E. B.; Gade, A.; Keek, L.; Kontos, A.; Lemasson, A.; Lunderberg, E.; Meisel, Z.; Noji, S.; Nunes, F. M.; Perdikakis, G.; Pereira, J.; Quinn, S. J.; Recchia, F.; Schatz, H.; Scott, M.; Simon, A.; Spyrou, A.; Stevens, J.; Stroberg, S. R.; Weisshaar, D.; Wheeler, J.; Wimmer, K.; Zegers, R. G. T.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA |
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Amer Physical Soc |
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English |
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2469-9985 |
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Notes |
WOS:000401655000003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3139 |
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Author |
Caballero-Folch, R. et al; Domingo-Pardo, C.; Agramunt, J.; Algora, A.; Rubio, B.; Tain, J.L. |
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Title |
beta-decay half-lives and beta-delayed neutron emission probabilities for several isotopes of Au, Hg, Tl, Pb, and Bi, beyond N=126 |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
95 |
Issue |
6 |
Pages |
064322 - 16pp |
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Abstract |
Background: There have been measurements on roughly 230 nuclei that are beta-delayed neutron emitters. They range from He-8 up to La-150. Apart from 210Tl, with a branching ratio of only 0.007%, no other neutron emitter has been measured beyond A = 150. Therefore, new data are needed, particularly in the region of heavy nuclei around N = 126, in order to guide theoretical models and help understand the formation of the third r-process peak at A similar to 195. Purpose: To measure both beta-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb, and Bi isotopes beyond N = 126. Method: Ions of interest were produced by fragmentation of a U-238 beam, selected and identified via the GSI-FRS fragment separator. A stack of segmented silicon detectors (SIMBA) was used to measure ion implants and beta decays. An array of 30 He-3 tubes embedded in a polyethylene matrix (BELEN) was used to detect neutrons with high efficiency and selectivity. A self-triggered digital system is employed to acquire data and to enable time correlations. The latter were analyzed with an analytical model and results for the half-lives and neutron-branching ratios were derived by using the binned maximum-likelihood method. Results: Twenty new beta-decay half-lives are reported for Au204-206, Hg208-211, Tl211-216, Pb215-218, and Bi218-220, nine of them for the first time. Neutron emission probabilities are reported for Hg-210,Hg-211 and Tl211-216. Conclusions: The new beta-decay half-lives are in good agreement with previous measurements on nuclei in this region. The measured neutron emission probabilities are comparable to or smaller than values predicted by global models such as relativistic Hartree Bogoliubov plus the relativistic quasi-particle random phase approximation (RHB + RQRPA). |
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Address |
[Caballero-Folch, R.; Calvino, F.; Cortes, G.; Gomez-Hornillos, M. B.; Riego, A.] Univ Politecn Cataluna, DFEN, INTE, E-08028 Barcelona, Spain, Email: rcaballero-folch@triumf.ca |
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Amer Physical Soc |
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English |
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2469-9985 |
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Notes |
WOS:000404022100001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3176 |
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Author |
n_TOF Collaboration (Wright, T. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement of the U-238(n,gamma) cross section up to 80 keV with the Total Absorption Calorimeter at the CERN n_TOF facility |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
96 |
Issue |
6 |
Pages |
064601 - 11pp |
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Keywords |
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Abstract |
The radiative capture cross section of a highly pure (99.999%), 6.125(2) grams and 9.56(5) x 10(-4) atoms/barn areal density U-238 sample has been measured with the Total Absorption Calorimeter (TAC) in the 185 m flight path at the CERN neutron time-of-flight facility n_TOF. This measurement is in response to the NEA High Priority Request list, which demands an accuracy in this cross section of less than 3% below 25 keV. These data have undergone careful background subtraction, with special care being given to the background originating from neutrons scattered by the 238U sample. Pileup and dead-time effects have been corrected for. The measured cross section covers an energy range between 0.2 eV and 80 keV, with an accuracy that varies with neutron energy, being better than 4% below 25 keV and reaching at most 6% at higher energies. |
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Address |
[Wright, T.; Billowes, J.; Ryan, J. A.; Ware, T.] Univ Manchester, Manchester, Lancs, England, Email: tobias.wright@manchester.ac.uk |
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Amer Physical Soc |
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English |
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2469-9985 |
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Notes |
WOS:000416848700005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3392 |
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Author |
n_TOF Collaboration (Lerendegui-Marco, J. et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
97 |
Issue |
2 |
Pages |
024605 - 21pp |
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Abstract |
The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA. |
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Address |
[Lerendegui-Marco, J.; Guerrero, C.; Quesada, J. M.; Cortes-Giraldo, M. A.; Praena, J.; Sabate-Gilarte, M.] Univ Seville, Dept Fis Atom Mol & Nucl, E-41012 Seville, Spain, Email: cguerrero4@us.es |
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Publisher |
Amer Physical Soc |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
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Notes |
WOS:000424190700001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3474 |
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